春季北黄海辽东半岛东部邻近海域溶解甲烷的分布、影响因素及海−气交换通量

Distributions, influencing factors and fluxes of dissolved methane in the eastern part of Liaodong Peninsula in the North Yellow Sea in spring

  • 摘要: 本文基于2022年5月现场调查,研究了北黄海辽东半岛东部邻近海域溶解甲烷(CH4)的分布、影响因素及海−气交换通量。结果表明,该海域溶解CH4浓度为3.2~11.2 nmol/L,饱和度为103%~364%,高值区位于鸭绿江口近岸海域,随着河口向海延伸,表层海水溶解CH4浓度逐渐减小,而底层海水溶解CH4浓度升高;鸭绿江冲淡水的输入致使近岸海域溶解CH4浓度显著升高,而沉积物有机质降解使得离岸海域底层海水溶解CH4浓度升高;该海域海−气CH4交换通量为0.7~61.1 μmol/(m2·d),是大气 CH4的源,近岸海域显著高于离岸海域。鸭绿江冲淡水的输入即使在平水期(5月)已经对邻近海域溶解CH4的影响非常显著,因此,河口等近岸海域海−气CH4交换通量的研究对于评估我国陆架边缘海对大气CH4的贡献至关重要。

     

    Abstract: Distributions, influencing factors and air-sea fluxes of methane (CH4) in the eastern part of Liaodong Peninsula in the North Yellow Sea were studied based on a field survey conducted in May 2022. Dissolved CH4 concentrations were 3.2~11.2 nmol/L, with the saturation of 103%~364%, showing an obvious decreasing trend in surface seawater and increasing trend in bottom seawater from inshore to offshore areas. The input of Yalu River resulted in a significant increase of dissolved CH4 in the inshore area, while dissolved CH4 in bottom water of the offshore area increased due to the degradation of organic matters in sediments. The studied area was an important source of atmospheric CH4 and the air-sea fluxes were 0.7~61.1 μmol/(m2·d), the inshore area is significantly higher than the offshore area. The input of Yalu River has significant effect on dissolved CH4 in the adjacent areas even in the normal water period. Future work should mainly focus on the investigation of the estuaries and other coastal waters to scientifically assess the air-sea CH4 fluxes in the marginal sea.

     

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