连云港田湾海域沉积物中放射性核素分布与沉积速率

Radionuclide distribution in sediments and sedimentary rates in the Tianwan sea area of Lianyungang

  • 摘要: 本文基于连云港田湾海域沉积物中放射性核素含量的测定结果,分析了表层沉积物中放射性核素含量的平面分布和柱状沉积物中放射性核素含量及垂向分布特征,并讨论了核素之间的内在关联和田湾近岸区的沉积速率。结果显示:(1)田湾海域表层沉积物类型基本为粉砂质黏土和黏土质粉砂,其中值粒径约为0.006 mm,平均黏土含量约为45%,属典型淤泥质海岸沉积物特征;(2)表层沉积物中某一放射性核素(210Pb、238U、228Ra、40K、226Ra、228Th、137Cs)比活度变化较大,但总体上处于相同水平;(3)210Pb、226Ra、238U和228Th垂向比活度范围分别为32.6~48.8 Bq/kg、17.6~33.3 Bq/kg、15.1~40.8 Bq/kg和40.31~86.9 Bq/kg,各核素含量随深度增加的变化规律有所不同;(4)柱状样中垂向上210Pb/226Ra活度比值为1.2~2.6,均值为1.5,210Pb明显过剩,且其过剩量与埋深有较明显的关系;(5)田湾附近50多年来的平均沉积速率为2.3 cm/a,60 cm以浅的沉积速率约为3.0 cm/a,60 cm以深的沉积速率约为1.0 cm/a;60 cm以浅的沉积速率较快,可能与近年来周边工程较多(田湾跨海大桥、取排水口、港区扩建等)有关。

     

    Abstract: Radionuclides in sediments of the Tianwan sea area were measured using the HPGe γspectrum method. Based on the data of sediments’ radionuclide content, the horizontal distribution of radionuclide content in surface sediments and the vertical distribution of radionuclide content in columnar sediments were analyzed, and the intrinsic correlation between the nuclides and the deposition rate in the near shore area of Tianwan were also discussed. The results showed that the surface sediments in the Tianwan sea area were basically silty clay and clayey silty sand, with an average median particle size of about 0.006 mm and an average clay content of about 45%, which are typical silty coastal sediments. Although the radioactive nuclide specific activities of 210Pb, 238U, 228Ra, 40K, 226Ra, 228Th, and 137Cs in surface sediment varied greatly, the horizontal level of individual radionuclide was similar. The range of vertical specific activity of 210Pb, 226Ra, 238U and 228Th was 32.6~48.8 Bq/kg, 17.6~33.3 Bq/kg, 15.1~40.8 Bq/kg and 40.3~86.9 Bq/kg, and each nuclide content changing with depth increase volatility rule was different. In the columnar sample, the vertical activity ratio of 210Pb/226Ra was between 1.2 and 2.6, with the mean value of 1.5. Excess of 210Pb was obvious in comparison with 226Ra and the excess was significantly related to the buried depth. Over the past 50 years, the average deposition rate near Tianwan was 2.3 cm/a, the deposition rate of column samples less than 60 cm was about 3.0 cm/a, and that of column samples greater than 60 cm was about 1.0 cm/a. deposition rate from 0 cm to 60 cm was relatively fast, which may be related to the influence of surrounding projects (Tianwan Cross-sea Bridge, drainage outlet, port expansion, etc.), and the deposition rate from 60 m to 100 cm was relatively slow and stable.

     

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